Bis(3-iodopropylammonium) lead iodide: Absorption (Kubelka−Munk)

Absorption (Kubelka−Munk)
Exciton binding energy, Eb ≈ 91 meV
Origin: experimental
Space group: P 2₁/c
X. Chen, H. Lu, K. Wang, Y. Zhai, V. Lunin, P. Sercel, and M. Beard, Tuning Spin-Polarized Lifetime in Two-Dimensional Metal−Halide Perovskite through Exciton Binding Energy, Journal of the American Chemical Society 143, 19438‑19445 (2021). doi: doi.org/10.1021/jacs.1c08514.
System description
Dimensionality: 2D n: 1
Sample type: powder
Related data
This data set is directly linked to other data sets: See all related data
X. Chen, H. Lu, K. Wang, Y. Zhai, V. Lunin, P. Sercel, and M. Beard, Tuning Spin-Polarized Lifetime in Two-Dimensional Metal−Halide Perovskite through Exciton Binding Energy, Journal of the American Chemical Society 143, 19438‑19445 (2021). doi: doi.org/10.1021/jacs.1c08514.

Extraction method: manual
Entry added on: Nov. 22, 2022, 12:37 a.m.
Entry added by: Harrison York Duke University
Last updated on: Nov. 29, 2022, 10:29 a.m.
Last updated by: Harrison York Duke University

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Data set ID: 2146 Did you find any mistakes or inconsistencies about this data? Send us a note and we'll have a look at it and send you a reply. Thanks!

Absorption (Kubelka−Munk)
Origin: experimental (T = 298.0 K)
R. Chakraborty, T. Sheikh, and A. Nag, Iodine−Iodine Interactions Suppressing Phase Transitions of 2D Layered Hybrid (I-(CH2)n‐NH3)2PbI4 (n = 2−6) Perovskites, Chemistry of Materials 34, 288‑296 (2022). doi: 10.1021/acs.chemmater.1c03492.
System description
Dimensionality: 2D n: 1
Sample type: single crystal

Starting materials: PbO, HI (57% (w/w) in water), H3PO2 (50% (w/w) in water)

Product: yellow plate-like crystals

Description: 5 mmol PbO was dissolved in a solution of 40 mL HI and 5 mL of H3PO2 by sonicating in an ultrasonic bath sonicator for 10 min. The solution is cooled to ∼278 K using an ice−water bath. In this solution, 10 mmol H2N-(CH2)3-OH is added dropwise. The solution is stirred using a magnetic stirrer and heated for 30 min in an oil bath maintained at 383 K. After 30 min, the heating and stirring are stopped, and the solution is kept undisturbed. After 12 hours, the precipitated crystals are separated by filtration with diethyl ether and dried in air.

Method: Diffuse reflectance spectroscopy

Description: The spectrum was recorded using a Shimadzu UV3600 plus UV−vis−NIR spectrophotometer with BaSO4 powder as a reference of 100% reflectance. The reflectance signal is converted to absorbance using the Kubelka−Munk function.

R. Chakraborty, T. Sheikh, and A. Nag, Iodine−Iodine Interactions Suppressing Phase Transitions of 2D Layered Hybrid (I-(CH2)n‐NH3)2PbI4 (n = 2−6) Perovskites, Chemistry of Materials 34, 288‑296 (2022). doi: 10.1021/acs.chemmater.1c03492.

Entry added on: Feb. 24, 2023, 10:44 a.m.
Entry added by: Rayan C Duke University
Last updated on: Feb. 24, 2023, 10:45 a.m.
Last updated by: Rayan C Duke University

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Data set ID: 2254 Did you find any mistakes or inconsistencies about this data? Send us a note and we'll have a look at it and send you a reply. Thanks!


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