Bis(2-bromoethylammonium) lead iodide: atomic structure

Atomic structure Verified
Origin: experimental (T = 173.0 (±2.0) K)
Space group: P n m a
Lattice parameters

Crystal system: orthorhombic

a:12.8543 (±0.0007) Å
b:20.7714 (±0.0013) Å
c:6.4866 (±0.0004) Å
α:90°
β:90°
γ:90°
Fixed parameters:
  • temperature = 173.0 (±2.0) K
A. Lemmerer and D. G. Billing, Effect of heteroatoms in the inorganic–organic layered perovskite-type hybrids [(ZCnH2nNH3)2PbI4], n = 2, 3, 4, 5, 6; Z = OH, Br and I; and [(H3NC2H4S2C2H4NH3)PbI4], CrystEngComm 12, 1290‑1301 (2010). doi: 10.1039/B917824D.
System description
Dimensionality: 2D n: 1
Sample type: single crystal

Starting materials: PbI2, HI, BrC2H4NH2·HBr

Product: Red crystals

Description: PbI2 (0.113 mmol; 0.052 g) was dissolved in 2 mL HI solution. Then BrC2H4NH2·HBr (0.376 mmol; 0.077 g) was added. The precipitate was dissolved at room temperature via ultrasound. The solution was then cooled in a fridge to 5 degrees Celsius, causing red crystals to precipitate.

Method: Single-crystal X-ray diffraction

Description: A Bruker SMART 1K CCD area detector diffractometer using Mo Kalpha radiation was used to measure SCXRD at 173 K. Omega-scans of width 0.3 degrees were used. The SAINT+ version 6.02 program was used for data reduction and the XPREP program was used for absorption corrections. SHELXS-97 was used to directly solve the structure. SHELXL-97 was used for refinement of the structure.

A. Lemmerer and D. G. Billing, Effect of heteroatoms in the inorganic–organic layered perovskite-type hybrids [(ZCnH2nNH3)2PbI4], n = 2, 3, 4, 5, 6; Z = OH, Br and I; and [(H3NC2H4S2C2H4NH3)PbI4], CrystEngComm 12, 1290‑1301 (2010). doi: 10.1039/B917824D.

Extraction method: Manually extracted from a publication
Entry added on: July 8, 2020, 12:13 a.m.
Entry added by: Andrew Levin NREL
Last updated on: July 4, 2022, 12:41 p.m.
Last updated by: Rayan C Duke University
Data correctness verified by:
  • Rayan C Duke University

Download data
Data set ID: 1176 Did you find any mistakes or inconsistencies about this data? Send us a note and we'll have a look at it and send you a reply. Thanks!

 

Atomic coordinates


Atomic structure Verified
Origin: experimental (T = 293.0 (±2.0) K, 293.0 (±2.0) K)
Space group: C2/c
Lattice parameters #1 - Phase 1: Space Group C2/c

Crystal system: monoclinic

a:9.1263 (±0.001) Å
b:9.1429 (±0.001) Å
c:21.45 (±0.002) Å
α:90°
β:98.65 (±0.001)°
γ:90°
Fixed parameters:
  • temperature = 293.0 (±2.0) K
S. Sourisseau, N. Louvain, W. Bi, N. Mercier, D. Rondeau, F. Boucher, J. Buzaré, and C. Legein, Reduced Band Gap Hybrid Perovskites Resulting from Combined Hydrogen and Halogen Bonding at the Organic−Inorganic Interface, Chemistry of Materials 19, 600‑607 (2007). doi: 10.1021/cm062380e.
Lattice parameters #2 - Phase 2: Space Group Pbnm

Crystal system: orthorhombic

a:6.4824 (±0.0003) Å
b:12.9046 (±0.0008) Å
c:21.1409 (±0.0016) Å
α:90°
β:90°
γ:90°
Fixed parameters:
  • temperature = 293.0 (±2.0) K
S. Sourisseau, N. Louvain, W. Bi, N. Mercier, D. Rondeau, F. Boucher, J. Buzaré, and C. Legein, Reduced Band Gap Hybrid Perovskites Resulting from Combined Hydrogen and Halogen Bonding at the Organic−Inorganic Interface, Chemistry of Materials 19, 600‑607 (2007). doi: 10.1021/cm062380e.
System description
Dimensionality: 2D n: 1
Sample type: single crystal

Starting materials: Acetonitrile, HI, Br(CH2)2NH2, PbI2

Product: Red plate-like crystals

Description: In 6:2:1 molar ratio HI, Br-(CH2)2-NH2, and PbI2 were added to an acetonitrile solution. It was stirred for a short time at room temperature, forming a clear and yellow solution. It was then held at room temperature and allowed to evaporate, leaving behind crystals of the perovskite after a few hours.

Method: Single-crystal X-ray diffraction

Description: A Bruker-Nonius KAPPA-CDD diffractometer using Mo Kalpha radiation was used to collect the SCXRD data. The Shelxl97 package was used to both solve and refine the structures.

S. Sourisseau, N. Louvain, W. Bi, N. Mercier, D. Rondeau, F. Boucher, J. Buzaré, and C. Legein, Reduced Band Gap Hybrid Perovskites Resulting from Combined Hydrogen and Halogen Bonding at the Organic−Inorganic Interface, Chemistry of Materials 19, 600‑607 (2007). doi: 10.1021/cm062380e.

Extraction method: Manually extracted from a publication
Entry added on: July 13, 2020, 7 p.m.
Entry added by: Andrew Levin NREL
Last updated on: July 4, 2022, 5:20 p.m.
Last updated by: Rayan C Duke University
Data correctness verified by:
  • Rayan C Duke University

Download data
Data set ID: 1329 Did you find any mistakes or inconsistencies about this data? Send us a note and we'll have a look at it and send you a reply. Thanks!

 

Atomic coordinates



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