Bis(hexylammonium) lead iodide: photoluminescence

Photoluminescence
Origin: experimental (T = 300.0 K)
E. P. Booker, T. H. Thomas, C. Quarti, M. R. Stanton, C. D. Dashwood, A. J. Gillett, J. M. Richter, A. J. Pearson, N. J. L. K. Davis, H. Sirringhaus, M. B. Price, N. C. Greenham, D. Beljonne, S. E. Dutton, and F. Deschler, Formation of Long-Lived Color Centers for Broadband Visible Light Emission in Low-Dimensional Layered Perovskites, JOURNAL OF THE AMERICAN CHEMICAL SOCIETY 139, 18632‑18639 (2017). doi: 10.1021/jacs.7b10223.
System description
Dimensionality: 2D n: 1
Sample type: powder

Starting materials: C6H16N, HI, PbI2, EtO2

Product: Powder of (C6H13NH3)2PbI4

Description: Prepare hexylammonium iodide salts via neutralization of HI with HA. Remove unreacted species by evaporation. Purify product by recrystallization in minimal diethyl ether/excess hexane and isolate via vacuum filtration. Prepare films by spin-coating or drop-casting solutions (prepared by dissolving HAI and PbI2 powders at a 2.5:1 molar ratio in a 1:0.34 volume ratio mixture of THF and methanol). Spin-coat films from solutions of 20 mg/mL at 2000 rpm for 30 s and anneal for 15 min at 70 °C.

Method: Photoluminescence spectra

Description: Steady-state photoluminescence emission spectra of spin-coated films on glass were measured at room temperature with a step size of 1 nm in an Edinburgh Instruments FLS980 fluorimeter by exciting with monochromated light with a 2 nm bandwidth at 480 nm.

E. P. Booker, T. H. Thomas, C. Quarti, M. R. Stanton, C. D. Dashwood, A. J. Gillett, J. M. Richter, A. J. Pearson, N. J. L. K. Davis, H. Sirringhaus, M. B. Price, N. C. Greenham, D. Beljonne, S. E. Dutton, and F. Deschler, Formation of Long-Lived Color Centers for Broadband Visible Light Emission in Low-Dimensional Layered Perovskites, JOURNAL OF THE AMERICAN CHEMICAL SOCIETY 139, 18632‑18639 (2017). doi: 10.1021/jacs.7b10223.

Extraction method: manually
Entry added on: July 29, 2022, 5:01 a.m.
Entry added by: Elisa Wade Albert-Ludwigs-Universität Freiburg
Last updated on: July 29, 2022, 5:01 a.m.
Last updated by: Elisa Wade Albert-Ludwigs-Universität Freiburg

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